Pressing the Print Screen button causes the Roblox client to freeze entirely, you can’t move the cursor or anything. You have to close the notification that you took a screenshot for it to work again (really annoying in fullscreen). If you press “Never See Again” on the notification the client only freezes for a portion of a second when you press Print Screen.
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Yep, been having this for over a year now, surprised it never got attention 
heres a related feature request
To add to this, the record feature does it and will sometimes just cause the client to close without warning
It’s not crashing, the screenshot popup sometimes just doesn’t get brought to the front.